题目: Toward Atomically Precise Heterogeneous Catalysis in Chemistry

报告人:李隽 教授， 清华大学

时间: 2020年12月2日（周三）15:00

地点: 化报厅

摘要:Catalysis science is essential for chemical industries, biological transformation, atmospheric processes, environment, energy, and human health. In recent years, heterogeneous single-atom catalysts (SACs) and single-cluster catalysts (SCCs) have aroused significant interest in the catalysis community [1-3]. In this talk, we will provide an overview and perspective of atomically precise heterogeneous catalysis via SACs and SCCs.

References: [1] (a) B.-T. Qiao, A.-Q. Wang, X.-F. Yang, L. F. Allard, Z. Jiang, Y.-T. Cui, J.-Y. Liu, J. Li, T. Zhang, "Single-Atom Catalysis of CO Oxidation Using Pt1/FeOx", Nature Chem. 2011, 3, 634−641.

(b) X.-F. Yang, A.-Q. Wang, B.-T. Qiao, J. Li, J.-Y. Liu, T. Zhang, "Single-Atom Catalysts: A New Frontier in Heterogeneous Catalysis", Acc. Chem. Res. 2013, 46, 1740-1748.

(c) A. Wang, J. Li, T. Zhang, “Heterogeneous Single-Atom Catalysis”, Nat. Rev. Chem. 2018, 2, 65-81.

[2] (a) J.-C. Liu, Y.-G. Wang, J. Li, "Toward Rational Design of Oxide-Supported Single Atom Catalysts: Atomic Dispersion of Gold on Ceria", J. Am. Chem. Soc. 2017, 139, 6190-6199.

(b) J.-C. Liu, Y. Tang, Y.-G. Wang, T. Zhang, J. Li, "Theoretical Understanding of the Stability of Single-Atom Catalysts", Natl. Sci. Rev. 2018, 5, 638-641.

[3] (a) X.-L. Ma, J.-C. Liu, H. Xiao, J. Li, "Surface Single-Cluster Catalyst for N2-to-NH3 Thermal Conversion", J. Am. Chem. Soc. 2018, 140, 46-49.

(b) J.-C. Liu, X.-L. Ma, Y. Li, Y.-G. Wang, H. Xiao, J. Li, "Heterogeneous Fe3 Single-Cluster Catalyst for Ammonia Synthesis via an Associative Mechanism", Nature Commun. 2018, 9, 1610.